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Photoinduced charge flow inside an iron porphyrazine complex
浏览: 发布日期:2019-11-08

Abstract

Tracking inorganic photochemistry with high resolution poses considerable challenges. Here, sub-picosecond electronic and structural motions and MLCT/d–d intersystem crossing in a cationic iron-porphyrazine are probed using ultrafast transient absorption, stimulated Raman spectroscopy, and quantum calculations. By delineating photoinduced energy relaxation, strategies for extending the lifetime of MLCT state are discussed.

Graphical abstract: Photoinduced charge flow inside an iron porphyrazine complex

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